Robert,
In order to change max item sizes you need to connect to Connect to Exchange Online PowerShell | Microsoft Docs. Once that is done you can view max item sizes with
Get-Mailbox testuser | fl mailboxplan,maxsendsize,maxreceivesize
This will set your O365 environment but it does not change existing user mailboxes
Get-MailboxPlan | Set-MailboxPlan -MaxSendSize 150MB -MaxReceiveSize 150MB
To change limits for all users
Get-Mailbox | Set-Mailbox -MaxReceiveSize 150MB -MaxSendSize 150MB
Once a cutover migration has been completed and it did not fail you cannot run it again because it will duplicate everything
In the case you have now I would complete the cutover migration so that users will use O365 from now on but do not uninstall Exchange Server 2010 yet from the SBS as we can try to export mail to pst files, see Export mailboxes from Exchange Server 2010 to pst files. Exporting may help you to retain the emails that were not migrated but exporting to pst files also has limitations, read Mailbox imports and exports in Exchange Server | Microsoft Docs
answered 01/15/2020 10:53